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Harrington, J. F., Milodowski, A. E., Graham, C. C., Rushton, J. C., Cuss, R. J. (2012) Evidence for gas-induced pathways in clay using a nanoparticle injection technique. Mineralogical Magazine, 76 (8) 3327-3336 doi:10.1180/minmag.2012.076.8.45

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Reference TypeJournal (article/letter/editorial)
TitleEvidence for gas-induced pathways in clay using a nanoparticle injection technique
JournalMineralogical Magazine
AuthorsHarrington, J. F.Author
Milodowski, A. E.Author
Graham, C. C.Author
Rushton, J. C.Author
Cuss, R. J.Author
Year2012 (December)Volume76
Issue8
PublisherMineralogical Society
DOIdoi:10.1180/minmag.2012.076.8.45Search in ResearchGate
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Mindat Ref. ID244348Long-form Identifiermindat:1:5:244348:9
GUID0
Full ReferenceHarrington, J. F., Milodowski, A. E., Graham, C. C., Rushton, J. C., Cuss, R. J. (2012) Evidence for gas-induced pathways in clay using a nanoparticle injection technique. Mineralogical Magazine, 76 (8) 3327-3336 doi:10.1180/minmag.2012.076.8.45
Plain TextHarrington, J. F., Milodowski, A. E., Graham, C. C., Rushton, J. C., Cuss, R. J. (2012) Evidence for gas-induced pathways in clay using a nanoparticle injection technique. Mineralogical Magazine, 76 (8) 3327-3336 doi:10.1180/minmag.2012.076.8.45
Abstract/NotesAbstractCorrosion, water radiolysis and microbial degradation will result in the generation of gas within repositories designed for the geological disposal of high-level radioactive waste. It is therefore crucial in the design of such facilities that the relevant mechanisms allowing gas migration through repository materials, both engineered barriers and clay-based candidate host rocks, are correctly identified. In Belgium, the Boom Clay represents a candidate host material for which the advective gas breakthrough characteristics and transport properties have been extensively tested and are well defined by numerous studies. The Boom Clay displays a significant capacity for self-sealing and both laboratory and field tests indicate that advective gas transport occurs not by visco-capillary flow, but instead through the formation of pressure-induced dilatant pathways. In this study, we present results from a gas injection test designed to demonstrate the presence of these features by injecting nanoparticulate tracers with helium gas into a sample of Boom Clay. The results provide conclusive evidence for the formation of transient, dilatant gas pathways within a candidate clay-based host rock. This technique provides a novel diagnostic tool for the identification of processes governing multi-phase flow, supporting robust long-term assessments of repository performance.


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